4.1 Significance of Welding Parameters
The analysis of variance (ANOVA) was carried out on the measured weld characteristics to determine the statistical significance of the welding parameters. All ANOVA tables are presented in Appendix A (Table 10) and include probabilities of significance (P), degrees of freedom (DOF), sum of squares (SS), variance ratios (F), and R2 values for each welding parameter. According to the statistical analysis reported by Mruczek et al. [6] and Shahverdi et al. [22], P values are used to determine the statistical significance of each of the welding parameters. A P value equal to or less than 0.05 indicates the parameter is statistically significant with 95% confidence. A P value of 0.25 corresponds to a 75% confidence level that the parameter is statistically significant for the weld characteristic. The P values for individual weld geometry results and micro-hardness values for the CGHAZ and WM are listed in Table 7, along with confidence levels. For 95% and 75% confidence levels, the significant welding parameters are highlighed in bold. For example, the significant welding parameters affecting reinforcement area (RA) are heat input of the trail electrode (HIT), voltage of the trail electode (VT) and bevel design (BD), all with a confidence level of 95%.
The effective contribution of each parameter depends on the sum of squares, which is the deviation from the total average value of population. The concept of the effective contribution is a fundamental term in ANOVA analysis and can be calculated by Eq. 5 [14].
$$\text{Ƥ}\text{%}=\frac{\text{S}{S}_{i}}{{SS}_{t}}\bullet 100\text{%}$$
5
where \(\text{Ƥ}\) is the effective contribution of each parameter to the response characteristics and \(\text{S}{S}_{i}\) and \({SS}_{t}\) are the sum of squares for each parameter and the total sum of squares, respectively. The contribution evaluates the importance of parameters on each weld characteristic and the WM and CGHAZ micro-hardness. The significant contributions for BW, AR, DIL, and SPR are shown in Fig. 6.
Overall voltage (lead + trail electrodes) and TS significantly influence BW, AR, and SPR, as shown in Fig. 6. It is generally accepted that a higher arc voltage leads to a wider arc length promoting the formation of a wide BW [23]–[25]. Thomas et al. [26] correlated TS with BW of heavy gauge strip and reported that a high TS reduces the filler metal per unit length of weld leading to a narrow weld. Specifically, a faster TS and lower V result in a shorter arc length and, as such, a smaller BW. The AR and SPR were calculated using Equations 2 and 3. Both geometric ratio results are significantly affected by VL and TS. An increasing TS results in a smaller BW due to the reduced heat input and reduced melted metal per unit length [25, 27]. Therefore, both AR and SPR are affected by voltage and TS, due to the change in BW. Dilution is defined as the ratio of the amount of adjacent metal melted to the total amount of fused metal. The amount of dilution is affected by two geometric results, PA and RA, as expressed in Eq. 4. There are two significant parameters, HIL and VT, that affect PA and RA. In this study, the polarity of the HIL is DCEP in the welding process producing a weld with good penetration [25, 28]. Therefore, a higher HIL increases the penetration depth leading to more dilution. Finally, it is common to minimize the amount of dilution since the amount of dilution affects the composition of the molten pool and the resultant mechanical properties in the welds [7, 29].
Figure 7 shows that the CWFS has the most dominant effect on the CGHAZ and WM micro-hardness profiles, since cold wire addition alters the local thermal cycle by absorbing the heat from the molten pool. Mohammadijoo et al. [30, 31] evaluated the effect of cold wire addition on heat input and hardness profile in the HAZ and they reported that increasing the CWFS leads to a higher hardness because of the faster cooling rate. In addition, the heat input and voltage may also contribute to the CGHAZ hardness profile since they can change the local thermal cycle and the size of the CGHAZ area. It is difficult to compare the effects of CWFS on hardness when other parameters are varied as well. Therefore, nonlinear relationship analysis between interactions of welding parameters and micro-hardness profiles in the CGHAZ and WM is necessary and is discussed in Subsection 4.2.
In Fig. 8, BD had the greatest effect on HRA, BTA, CGHAZ area, and RA. In order to understand the effect of BD, the 16 measurements of RA, HRA, BTA, and CGHAZ area were plotted against two bevel specifications separately, as shown in Fig. 9. The BD with a wider bevel area had lower RA and HRA, and increased BTA and CGHAZ area. This means that smaller and shallower reinforcement regions were produced for the larger bevel angle.
According to the study on the influence of bevel angle on heat transfer and fluid flow in the welding pool, published by Chen et al. [32], increasing the bevel angle from 60° to 90° resulted in more liquid metal flowing downward. This means that increased bevel angle promotes heat transfer from the top to the bottom of the weld leading to full penetration. Huang et al. [33] also studied the effect of groove angle on weld depth in tungsten inert gas (TIG) welding by analyzing the current density and arc pressure. When the groove angle was increased, the current density and arc pressure were elevated at the groove bottom position, because of the concentrated arc heat input and stronger electromagnetic force at the bottom region of the high groove angle in comparison to the low groove angle [33]. This phenomenon indicates that there is a smaller RA in the wider BD than the shallower BD due to the achievement of full penetration.
The formation of a larger CGHAZ area in the deep BD than in the shallow BD is supported by Chen’s simulation study of thermal cycles in the molten pool. The finding showed that the width of the overheated zone (1100°C − 1500°C) increased when the bevel angle changed from 60° to 90°, which promoted the formation of a coarse grain structure. The reason for this phenomenon is that the arc and molten metal contacted a larger area when the bevel angle was larger, so that the solid metal phase easily conducted more heat to expand the overheated zone [32].
The BD had a smaller effect on the weld geometry (SPR and AR) and dilution than HI, V and TS, as shown in Fig. 6. The values of SPR and AR were calculated from the BW. The smaller effect of BD on the BW can be explained in terms of the main liquid metal flow pattern and surface tension in the molten pool. The main flow pattern of liquid metal in the molten pool is liquid metal flowing upward along the boundary of the molten pool and colliding at the top of the weld, whereupon the liquid metal changes direction and descends into the pool [32].
The main flow pattern of liquid metal and surface tension are governed the BW and they are affected by active elements, such as O, S, Si, and Ni, dissolved in the liquid mixture metal [32, 34]. The BW is controlled by the surface tension force since it pulls liquid metal towards the center of the weld pool, which is varied by the concentration of the active elements. Another study reported that bead width depends on the concentration of surface active elements and the local temperature profile [35]. In this study, the composition of the base metal X70 steel, the electrodes, and the granular flux were uniform and identical for all 16 fabricated weldments. This means that the main flow pattern, surface tension, and BW were not altered even for different bevel angles and bevel depths. Therefore, the BD had little influence on the weld geometry ratio.
4.2 Nonlinear Relationship of CWTSAW
Three order multiple regression (TOMR) was used to analyze the nonlinear relationship of controllable variables and the response factors. The empirical equations were developed using Minitab 18 with the form in Eq. 6.
$$\text{y}= {C}_{0}+\sum _{i=1}^{7}\left({C}_{i}\bullet {x}_{i}\right)+\sum _{i=1}^{7}\left({C}_{ii}\bullet {x}_{i}^{2}\right)+\sum _{i=1}^{7}\sum _{i>j}^{7}\left({C}_{ij}\bullet {x}_{i}\bullet {x}_{j}\right)+\sum _{i=1}^{7}\left({C}_{iii}\bullet {x}_{i}^{3}\right)+\sum _{i=1}^{7}\sum _{j>i}^{7}\sum _{k>j}^{7}\left({C}_{ijk}\bullet {x}_{i}\bullet {x}_{j}\bullet {x}_{k}\right)$$
6
where y is the response factor (geometry characteristics and micro-hardness profile) which was predicted by the controllable variable \({x}_{i}\)(welding parameters and different interactive combinations); \({C}_{i}\), \({C}_{ii}\), \({C}_{ij}\), \({C}_{iii}\), and \({C}_{ijk}\) are the coefficients. In this study, the confidence level of TOMR in Minitab 18 was set at 90% which means that any controllable variables with a P value less than or equal to 0.1 are statistically significant and considered as predictors in empirical equations. For example, 8 predictors in the CGHAZ micro-hardness TOMR equation from a total of 72 possible predictors (individual welding parameters and interactions) were considered which resulted in a good fit.
CGHAZ micro-hardness = 112 + 1.86∙ CWFS + 298∙ HIL − 13.31∙ VL + 1.44∙ TS -0.0327∙ CWFS2-5.89∙ HIL∙ TS + 0.264∙ VL∙ TS + 0.000169∙ CWFS3 (7)
Of particular note is that squared and cubed predictors are only associated with CWFS in the CGHAZ micro-hardness equation. This appears to be the dominant effect contributed by cold wire addition in comparison with other TOMR equations. The other TOMR equations for HRA, RA, CGHAZ area, SPR, and WM micro-hardness are shown in Appendix A.
The calculated values for HRA, RA, CGHAZ area, micro-hardness of the CGHAZ, and WM are plotted against the observed values in Fig. 10. To validate each equation, three (3) complementary tests were conducted and are included in Fig. 10 (triangles). The weld table for these complementary tests is shown in Table 4. Overall, the range of R2 values is from 81.6–97.9% and the geometric characteristics of the three complementary tests with the varied welding parameters levels show good correlation with the observed values (Fig. 10).
4.3 Optimized Levels of CWTSAW
The S/N ratio was utilized to determine the optimized levels for each welding parameter. The welding parameters were categorized by two quality requirements, which are “lower-the-better” and “higher-the-better”, respectively. AR, BTA, APR, and BW are included in the “higher-the-better” quality requirements. DIL, CGHAZ area, HRA, and RA are included in the “lower-the-better” quality requirements. The S/N ratio analysis was not conducted on the micro-hardness profiles since there is not agreement on which approach is better. The S/N ratio was calculated using Equations 8 and 9 [16].
$${{\eta }}_{ \left(\text{l}\text{o}\text{w}\text{e}\text{r}-\text{t}\text{h}\text{e}-\text{b}\text{e}\text{t}\text{t}\text{t}\text{e}\text{r}\right)}= -10{\text{l}\text{o}\text{g}}_{10}\left(\frac{1}{n}\sum _{i=1}^{n}{y}_{ij}^{2}\right)$$
8
$${{\eta }}_{ \left(\text{h}\text{i}\text{g}\text{h}\text{e}\text{r}-\text{t}\text{h}\text{e}-\text{b}\text{e}\text{t}\text{t}\text{t}\text{e}\text{r}\right)}= -10{\text{l}\text{o}\text{g}}_{10}\left(\frac{1}{n}\sum _{i=1}^{n}\frac{1}{{y}_{ij}^{2}}\right)$$
9
where \({\eta }\) is the S/N value, \({y}_{ij}\) is the experimental value of the \(i\)th response characteristic in the \(j\)th test, and \(n\) is the number of tests.
A higher average S/N ratio value representing a given level of the weld parameter resulted in an optimal effect on the geometric characteristics, since higher S/N values mean lower noise effects [15, 36]. A weld parameter level with a higher S/N value is considered as the optimized parameter level, which results in an optimal effect on the geometric characteristics. The calculated S/N ratio values for the weld characteristics are shown in Appendix A (Table 11). Based on the calculated S/N ratio values, the optimized levels for the CWTSAW parameters are summarized (Table 8). Overall, the optimal geometric characteristics are achieved using optimized levels of CWTSAW parameters; i.e., 1.6 kJ/mm for HIL (level 1), 1.3 kJ/mm for HIT (level 1), 21.2 mm/s for TS (level 1), and 25mm2 for BD (level 2).
4.4 Comparison of TSAW and CWTSAW
Two heavy gauge X70 welds were produced by conventional tandem submerged arc welding (TSAW) and cold wire TSAW (CWTSAW) processes. Then, a comparison in terms of average micro-hardness and the phase fraction of MA constituents in the CGHAZ of TSAW and CWTSAW weld was undertaken. The weld testing conditions are shown in Table 9. The HIL, HIT, VL, VT, TS ,and BD for both the TSAW and CWTSAW weld are identical and only the CWFS is varied.
The strategy of micro-hardness measurement followed the schematic description in Fig. 4. Figure 11 shows that the average micro-hardness values measured in the CGHAZ of the TSAW and CWTSAW welds. The hardness is higher for the CGHAZ of the TSAW weld than for the CWTSAW weld. The lower hardness distribution in the CGHAZ of CWTSAW weld is closely related to the microstructure modification due to heat reduction by heat consumption of the cold wire addition.
Optical and SEM SE micrographs of MA constituents in the CGHAZ of TSAW and CWTSAW samples are shown in Fig. 12. The MA constituents appear as shiny white features in the optical and SEM images after etching with the modified LePera’s etchant [19]. White linear segments are visible in the SEM images, since some of the MA constituents were formed at the grain boundaries (Fig. 12b and d). The MA fractions from the optical micrographs (Fig. 12a and b) are 5.3% (0.2%) and 2.8% (0.1%) for the TSAW and CWTSAW welds, respectively. The MA fractions in the CGHAZ determined from the SEM micrographs are 5.7% (0.2%) and 3.3% (0.2%) for TSAW and CWTSAW samples, respectively. The values in the brackets are one standard deviation. The trend for the MA phase fraction in the CGHAZ for both welds is consistent. In terms of the morphology of MA constituents, the MA regions in the TSAW sample from both optical and SEM SE micrographs are mainly massive and the MA constituents of the TSAW sample are more elongated and larger than those in the CWTSAW sample. The MA features in the CWTSAW sample are finer and more dispersed than those in the TSAW sample.
The CWTSAW samples have lower MA fractions with fine and dispersed MA constituents (Fig. 12c and d). The average micro-hardness in the CGHAZ of TSAW samples is higher than that in the CWTSAW sample, which can be correlated with the higher MA volume fraction and the different MA morphology (blocky and elongated) in the TSAW sample. Luo et al. [37] and Mohammadijoo et al. [38, 39] analyzed the morphology of martensite-austenite (MA) constituents in the CGHAZ with respect to the fracture toughness. They reported similar findings that denser MA regions with elongated MA constituents were formed at prior austenite grain (PAG) boundaries, which resulted in localized brittle zones (LBZs). The formation of LBZs can cause initiation and propagation of cleavage fracture at the PAG boundaries in the HAZ, deteriorating the fracture toughness. There are elongated MA constituents and a higher overall MA fraction in the CGHAZ of the TSAW sample than in the CWTSAW sample. This can be interpreted as the reason for the higher hardness in the CGHAZ of the TSAW samples.