We investigated the nucleation of Ga droplets on exact GaAs(111)A substrates in the view of their use as the seeds for the self-assembly droplet epitaxial quantum dots. A small critical cluster size of 1-2 atoms characterizes the droplet nucleation. Low values of the Hopkins-Skellam index (as low as 0.35) demonstrate a high degree of a spatial order of the droplet ensemble. Around 350 °C the droplet size distribution becomes bimodal. We attribute this observation to the interplay between the local environment and the limitation to the adatom surface diffusion introduced by the Ehrlich-Schwöbel barrier at the terrace edges.

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The full text of this article is available to read as a PDF.
No competing interests reported.
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Posted 03 Feb, 2021
On 19 Feb, 2021
Received 14 Feb, 2021
On 05 Feb, 2021
Invitations sent on 05 Feb, 2021
On 05 Feb, 2021
On 05 Feb, 2021
On 05 Feb, 2021
On 03 Feb, 2021
Posted 03 Feb, 2021
On 19 Feb, 2021
Received 14 Feb, 2021
On 05 Feb, 2021
Invitations sent on 05 Feb, 2021
On 05 Feb, 2021
On 05 Feb, 2021
On 05 Feb, 2021
On 03 Feb, 2021
We investigated the nucleation of Ga droplets on exact GaAs(111)A substrates in the view of their use as the seeds for the self-assembly droplet epitaxial quantum dots. A small critical cluster size of 1-2 atoms characterizes the droplet nucleation. Low values of the Hopkins-Skellam index (as low as 0.35) demonstrate a high degree of a spatial order of the droplet ensemble. Around 350 °C the droplet size distribution becomes bimodal. We attribute this observation to the interplay between the local environment and the limitation to the adatom surface diffusion introduced by the Ehrlich-Schwöbel barrier at the terrace edges.

Figure 1

Figure 2

Figure 3

Figure 4

Figure 5

Figure 6

Figure 7

Figure 8
The full text of this article is available to read as a PDF.
No competing interests reported.
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