3.1 Temporal analysis
Figure 2 shows the trend of the number of CCUS or CCS literature published in China and the United States during 2000–2022, and it can be seen that the technology shows an overall upward trend. Combined with the characteristics and laws of this technology development, this paper divides the development trend into three stages: the first stage is the slow growth stage (2000–2008), the second stage is the rapid rise stage (2009–2018), and the third stage is the booming stage (2019-Present). Figure 2 shows that the amount of literature on CCUS is less in the first phase (2000–2008). The United States published 63 articles, accounting for 2.52% of the total publications, while China published 4 papers, accounting for only 0.16% of the total. The first Chinese literature on CCUS was published in 2004. It shows that the United States is earlier than China regarding CCUS research. In the second phase (2009–2018). The United States published 813 articles, accounting for 32.55% of the total number of publications. China published 609 papers, accounting for 24.38% of the total number of publications. Both Chinese and US CCUS technologies have developed rapidly during this period. Among them, the trend of CCUS technology in the United States is increasing first and then stable, while China is in a state of rapid increase all the time. And in 2016, China surpassed the United States for the first time. The third phase is (2019-Present). The United States published 426 articles, accounting for 17.05% of the total publications, while China published 583 papers, accounting for 23.34% of the total publications. It can be seen that Chinese CCUS technology has been growing rapidly in this phase. In 2019, the Chinese government proposed to achieve carbon peaking by 2030 and a carbon neutrality target by 2060. CCUS technology, as one of the critical emission reduction technologies for carbon neutrality, has more Chinese scholars started to research CCUS technology. In 2021, the United States returned to the Paris climate agreement and pledged to achieve net-zero emissions by 2050. The 26th United Nations Climate Change Conference (COP 26) was held in the same year. As the international community pays more and more attention to the net-zero emission target, CCUS technology is rapidly developing, the number of literary publications about this technology will increase in the future, and the research about CCUS technology will usher in an essential window.
3.2 Analysis of the distribution of journals and academic fields
3.2.1 Analysis of journal distribution
Based on the subject classification of the web of science database. This study examines the field of CCUS technology in China and the United States from 2000–2022 through the distribution of literature by subject categories and journals. From the perspective of journal distribution, the top 15 journals with a total of 1138 articles (45.6% of the total publications) were selected for analysis (Table 1). The remaining 1360 articles were distributed in 448 journals, which are not discussed in this paper due to the small number of papers issued. Table 1 shows the top 15 journals regarding the number of publications and citation attributes for 2000–2022. These are well-known energy, environmental science, atmospheric science, and chemical chemistry journals. Table 1shows that the International Journal of Greenhouse Gas Control has the highest number of publications, with 322 articles, accounting for 12.89% of the total number of articles published. Followed by Applied Energy (120, 4.8%), Energy (90, 3.6%), and Environmental Science & Technology (88, 3.52%). Among the 15 most published journals, Energy & Environmental Science has the highest impact factor of 39.71. In addition, it has an average number of citations per publication of 145.57, ranking first among all journals. It shows that these journals have a tremendous academic influence. It can also be seen that these journals show a greater interest in the study of CCUS technology and are more essential journals in this field.
Rank
|
Journal
|
TP
|
R (%)
|
IF
|
TC
|
TC/TP
|
Table 1
Top15 most productive journals during 2000–2022
1
|
International Journal of Greenhouse Gas Control
|
322
|
12.89
|
4.4
|
7636
|
23.71
|
2
|
Applied Energy
|
120
|
4.80
|
11.47
|
4495
|
37.46
|
3
|
Energy
|
90
|
3.60
|
8.86
|
2467
|
27.41
|
4
|
Environmental Science & Technology
|
88
|
3.52
|
2.52
|
5730
|
65.11
|
5
|
Energy Policy
|
80
|
3.20
|
7.76
|
3921
|
49.01
|
6
|
Journal of Cleaner Production
|
72
|
2.88
|
11.08
|
2093
|
29.07
|
7
|
Greenhouse Gases-Science and Technology
|
67
|
2.68
|
2.52
|
808
|
12.06
|
8
|
Energy & Fuels
|
49
|
1.96
|
4.65
|
925
|
18.88
|
9
|
Industrial & Engineering Chemistry Research
|
48
|
1.92
|
4.33
|
1554
|
32.38
|
10
|
Energies
|
43
|
1.72
|
3.25
|
371
|
8.63
|
11
|
Climatic Change
|
36
|
1.44
|
5.17
|
1915
|
53.19
|
12
|
Energy Conversion and Management
|
32
|
1.28
|
11.53
|
620
|
19.38
|
13
|
Energy Economics
|
31
|
1.24
|
9.25
|
1026
|
33.10
|
14
|
Energy & Environmental Science
|
30
|
1.20
|
39.71
|
4367
|
145.57
|
15
|
Chemical Engineering Journal
|
30
|
1.20
|
16.74
|
677
|
22.57
|
Note: TP indicates the total number of articles published in the journal. IF indicates the journal impact factor. R (%) means the proportion of literature published in the journal to the total number of papers. TC indicates the total number of citations. TC/TP indicates the average number of citations per publication. |
3.2.2 Analysis of discipline distribution
From the perspective of disciplinary distribution, during 2000–2022, the CCUS in China and the United States are mainly clustered in 10 disciplinary areas, namely Engineering, Energy and Fuels, Environmental Science and Ecology, Science and Technology, Chemistry, Materials Science, Thermodynamics, Business and Economics, Geology, Meteorology and Atmospheric Sciences, and other topics. The distribution of literature disciplines shows that CCUS technology involves multidisciplinary fields. Among them, the engineering category accounted for 23.9% of the total articles issued and was first. Energy and Fuels, Environmental Science and Ecology for 21.49%, 12.07%, and 2.55%, respectively (Fig. 3). The research related to CCUS technology can be seen in engineering, environmental science, atmospheric science, business and economics, ecology, and energy. It can be seen that CCUS technology as a technology portfolio involves a wide range of disciplinary fields and has multidisciplinary cross-fertilization characteristics. It has received increasing attention from scholars with different disciplinary backgrounds.
3.3 Co‑institution network analysis
Table 2 shows the top 20 institutions in the United States and China regarding the number of articles published on CCUS topics from 2000 to 2022. In issuing institutions, there are 20 institutions with more than 37 articles, including 11 from China and 9 from the United States. These institutions have published 1197 articles, accounting for 47.92% of the total number of publications, indicating that they have solid scientific capabilities in the field of CCUS and have gathered many outstanding scientific scholars and teams. Comparing the number of articles published in China and the United States, it can be found that the Chinese Acad Sci has published the most papers, with 180 pieces (7.21%) ranking first in both institutions. Followed by Tsinghua University with 112 articles (4.48%), and Carnegie Mellon Univ of the United States organized the third. A total of 84 pieces (3.36%) were published. Although more articles were published in the United States than in China during 2000–2022, United States research institutions on CCUS did not rank first. This result indicates China's importance and outstanding contribution to research in CCUS-related fields.
Carnegie Mellon Univ ranked first in total article citations with 6580 citations. It was followed by Univ Calif Berkeley (3854) and Tsinghua Univ (3750), and Chinese Acad Sci (3695) in China. Other institutions with more than 2000 citations include MIT, Stanford Univ, and Princeton Univ. These institutions have a high level of scientific research. Undeniably, the United States, as one of the first countries to study CCUS technology, profoundly influences the CCUS field. In addition, in terms of cooperation intensity, Chinese Acad Sci inter-institutional linkage intensity reached 223, ranking first. Tsinghua University (117), and Univ Chinese Acad Sci (84), indicate that these institutions have some teamwork, but on the whole, the cooperation intensity of 14 institutions is less than 70. Others that have yet to be counted are lower. This is sufficient to show that the power of inter-institutional collaboration still needs to be further strengthened.
Rank
|
Institution
|
Country
|
TP
|
TC
|
AC (%)
|
TLS
|
Table 2
Top 20 institutions in China and the United States by number of publications
1
|
Chinese Acad Sci
|
China
|
180
|
3695
|
7.21
|
223
|
2
|
Tsinghua Univ
|
China
|
112
|
3750
|
4.48
|
117
|
3
|
Carnegie Mellon Univ
|
USA
|
84
|
6580
|
3.36
|
48
|
4
|
MIT
|
USA
|
79
|
3617
|
3.16
|
59
|
5
|
Univ Texas Austin
|
USA
|
66
|
1601
|
2.64
|
71
|
6
|
China Univ Petr
|
China
|
61
|
805
|
2.44
|
51
|
7
|
Univ Calif Berkeley
|
USA
|
60
|
3854
|
2.40
|
76
|
8
|
Stanford Univ
|
USA
|
49
|
3137
|
1.96
|
78
|
9
|
Princeton Univ
|
USA
|
49
|
2772
|
1.96
|
51
|
10
|
Univ Chinese Acad Sci
|
China
|
48
|
789
|
1.92
|
84
|
11
|
China Univ Min&Technol
|
China
|
48
|
725
|
1.92
|
43
|
12
|
North China Elect Power Univ
|
China
|
47
|
601
|
1.88
|
65
|
13
|
Tianjin Univ
|
China
|
47
|
995
|
1.88
|
43
|
14
|
Dalian Univ Technol
|
China
|
42
|
545
|
1.68
|
22
|
15
|
China Univ Geosci
|
China
|
39
|
563
|
1.56
|
66
|
16
|
Los Alamos Natl Lab
|
USA
|
38
|
1210
|
1.52
|
15
|
17
|
Beijing Inst Technol
|
China
|
37
|
833
|
1.48
|
19
|
18
|
Zhejiang Univ
|
China
|
37
|
1199
|
1.48
|
11
|
19
|
US DOE
|
USA
|
37
|
765
|
1.48
|
9
|
20
|
Columbia Univ
|
USA
|
37
|
1904
|
1.44
|
47
|
Note: TP indicates the total number of papers published. TC indicates the total number of citations. AC (%) represents the institution's contribution rate. TLS represents the full strength of ties between institutions. |
Meanwhile, as shown in Fig. 4. The number of articles published by the top six institutions in China and the United States offers a fluctuating growth trend, especially after 2005, when it started to grow faster. Chinese institutions overtook U.S. institutions around 2010. Three top 6 institutions are from China: Chinese Acad Sci, Tsinghua University, and China Univ Petr, and three from the US: Carnegie Mellon Univ, MIT, and Univ Texas Austin. Among them, Chinese Acad Sci had the fastest growth from 2011–2021, with 160 publications, accounting for 88.9% of the total publications of this institution. Chinese Acad Sci was also one of the first institutions to enter the field of CCUS-related research and published the first academic paper on CCUS technology research in China in 2004. It shows that the institution is at the forefront of CCUS research. As a world-renowned university, Tsinghua University has strong basic strength in scientific research. China Univ Petr, a famous university in the field of petroleum, has a particular influence on the engineering application of CCUS technology. From the figure, the research results related to CCUS technology were published by Carnegie Mellon Univ and MIT in 2001, respectively. And they have been in the leading position during 2000–2010 and keep rising at a specific rate. As the world's top academic institutions, they have some influence in the field of CCUS. However, the development in CCUS research is slower compared to China.
As the most important research institutions and universities in China and the U.S., These institutions have published very influential articles in CCUS-related fields, which have extensively promoted research in CCUS-related areas in both countries. In the future, both countries will have great potential for cooperation and development in CCUS technology development and innovation, large-scale promotion and application, and talent training.
3.4 Co‑author network analysis
Authors are the main body of scientific research, and the number of publications and citation attributes is commonly used to measure authors' research ability and academic influence. Author collaboration networks can clarify the core figures in scientific research fields and the collaboration and cross-citation relationships among different scholars. In this paper, we used VOSviewer software to map the knowledge of authors and teams in the field of CCUS in China and the United States during 2000–2022 (Fig. 5). This paper counted the information of the top 20 authors in terms of several publications as shown in Table 3. The ranking is based on the total number of publications by the authors. As can be seen from Table 3, among the top 20 authors in terms of the number of publications, there are 10 Chinese and 10 American scholars, and the top 5 authors in the CCUS research field in the United States are Rubin ES, Middleton RS, Zhai HB, Herzog HJ, and Bielicki JM. The top 5 authors in the field of CCUS research in China are Zhang X, Li Q, Li XC, Song YC, and Deng S. Rubin ES from Carnegie Mellon University published the most articles. There are 29 publications. This was followed by Middleton RS from Los Alamos Natl Lab and Carbon Solut LLC, with 28 publications. In fourth place is Zhang X from Minist Sci & Technol Most and Li Q from the Institute of Rock and Soil Mechanics in China, with 24 publications. In fifth place is Li XC, also from the Institute of Rock and Soil Mechanics in China, with 22 publications. Regarding the number of citations, Professor Rubin ES, also from the United States, ranked first with 2766 citations. They were followed by Herzog HJ (Massachusetts Institute of Technology, 1324), van Vuuren DP (Utrecht University, 1171), Middleton RS (Los Alamos Natl Lab and Carbon Solut LLC, 1138), Benson SM (Stanford University, 936), all from the United States. Li Q is China's most frequently cited scholar (Institute of Rock and Soil Mechanics, CAS, 724). It can be seen that American scholars have a more significant influence in the field of CCUS.
Regarding the H-index, Professor Van Vuuren, DP from Utrecht University in the United States, had the highest H-index of 93. The scholar's research interests focus on climate change, environmental science, and global sustainable development, and he has published a series of academic results (Biermann et al. 2022, Schweizer et al. 2020). Professor Wei YM (73) from the Beijing Institute of Technology in China is second. His research interests are energy and environmental policy (Kang et al. 2021, Li et al. 2022). Second, Professor Song YC from the Dalian University of Technology in China, whose H-index is 53, mainly focuses on carbon dioxide sequestration and resource utilization (Cheng et al. 2022, Liu et al. 2022a). And Professor Michael A. C from Princeton University in the United States, whose H-index reached 50. He has made significant contributions to flow in porous media, carbon storage, and numerical methods. Leon C (47) from the University of Maryland in the USA is in fifth place. His research interests are climate change, energy technology selection, and integrated assessment modeling. He is also currently the lead author of the IPCC Sixth Assessment Report Coordination (Ou et al. 2021, Yu et al. 2019). It can be found that both Chinese and American scholars have made significant contributions to the field of CCUS research. Still, American scholars have more significant academic influence between China and the United States.
Rank
|
Author
|
Institution
|
country
|
TP
|
TC
|
TLS
|
H-index
|
Table 3
The top 20 authors in terms of number of articles published in China and the USA
1
|
Rubin ES
|
Carnegie Mellon University
|
USA
|
29
|
2766
|
21
|
31
|
2
|
Middleton RS
|
Los Alamos Natl Lab and Carbon Solut LLC
|
USA
|
28
|
1138
|
51
|
19
|
3
|
Zhang X
|
Minist Sci & Technol Most
|
China
|
24
|
593
|
61
|
15
|
4
|
Li Q
|
Institute of Rock and Soil Mechanics, CAS
|
China
|
24
|
724
|
26
|
25
|
5
|
Li XC
|
Institute of Rock and Soil Mechanics, CAS
|
China
|
22
|
318
|
38
|
24
|
6
|
Zhai HB
|
Carnegie Mellon University
|
USA
|
18
|
689
|
15
|
19
|
7
|
Herzog HJ
|
Massachusetts Institute of Technology
|
USA
|
17
|
1324
|
16
|
23
|
8
|
Song YC
|
Dalian University of Technology
|
China
|
17
|
251
|
49
|
53
|
9
|
Deng S
|
Tianjin University
|
China
|
16
|
340
|
39
|
29
|
10
|
Wei YM
|
Beijing Institute of Technology
|
China
|
15
|
309
|
24
|
73
|
11
|
Li Z
|
Tsinghua University
|
China
|
15
|
509
|
24
|
43
|
12
|
Bielicki JM.
|
The Ohio State University
|
USA
|
15
|
635
|
23
|
23
|
13
|
Chen WY
|
Tsinghua University
|
China
|
14
|
682
|
8
|
27
|
14
|
van Vuuren DP
|
Utrecht University
|
USA
|
13
|
1171
|
43
|
93
|
15
|
Michael A. C
|
Princeton University
|
USA
|
13
|
614
|
11
|
50
|
16
|
Zhu L
|
Nanjing University of Information Science & Technology
|
China
|
13
|
53
|
29
|
27
|
17
|
Fan JL
|
China University of Mining & Technology, Beijing
|
China
|
13
|
283
|
39
|
28
|
18
|
Leon C
|
University of Maryland
|
USA
|
12
|
831
|
34
|
47
|
19
|
Benson SM
|
Stanford University
|
USA
|
12
|
936
|
2
|
36
|
20
|
Wilson EJ
|
Dartmouth College
|
USA
|
11
|
325
|
15
|
23
|
Note: TP indicates the total number of papers published. TC indicates the total number of citations. TLS represents the total link strength among authors. The H-index indicates that a researcher has at most H papers cited at least H times each. The higher the h-index, the more influential his papers are. |
Fig. 5 shows the critical scholars and major collaborative networks in the field of CCUS technology in China and the United States during 2000-2022. For example, Li XC and Li Q from the Institute of Rock and Soil Mechanics, CAS, and Wang YS from China Shenhua Group Corporation have formed a collaborative team to study geological storage and utilization of CO2, carbon neutral theory, technology, and engineering applications (Wang et al. 2021, Xu et al. 2019). A collaborative group, mainly consisting of Song YC from the Dalian University of Technology, focuses on new technologies for CO2 resource utilization and oil and gas extraction (Lu et al. 2022). Another group of collaborators mainly consists of Deng S from Tianjin University, focusing on CO2 capture technology (Li et al. 2021). In addition, Fan, JL, and Zhang X have contributed to the CCUS source-sink matching model (Fan et al. 2021) and LI Z to CO2 capture (Yang et al. 2022).
As seen in Fig. 5b, the United States CCUS research area collaboration teams are clustered in the following groups. The research team of Professor Rubin ES from Carnegie Mellon University focuses on CCS economic evaluation and policy (Roussanaly et al. 2021, Rubin et al. 2015). A research group consisting of Middleton RS from Los Alamos Natl Lab and Carbon Solut LLC has made contributions to CCS energy system optimization, numerical simulation, and fundamental architecture research (Middleton &Bielicki 2009, Middleton &Yaw 2018). Another collaborative group is composed of Prof. van Vuuren DP from Utrecht University. As described earlier, this scholar contributes significantly to studying climate change and global sustainability. This shows the efforts and contributions of many scholars and teams in the field of CCUS in China and the United States during the period 2000-2022. They are the most productive and influential authors and groups in the field of CCUS research.
Similarly, the number of highly cited papers is a crucial indicator of impact. Usually, the more awarded a piece is, the more recognized it is by the academic community. Table 4 shows the top 10 highly cited articles in the field of CCUS between China and the United States during 2000–2022, the United States has 7 out of 10 studies, and China has only 3. It can be seen that there is a gap between China and the United States in the field of CCUS, and the United States has more influence in CCUS.
Author
|
TC
|
Journal
|
Country
|
Research direction
|
Table 4
Top 10 highly cited articles in the CCUS field in the US and China from 2000 to 2022
Rao and Rubin (2002)
|
1334
|
Environmental Science & Technology
|
USA
|
Engineering; Environmental Sciences & Ecology
|
McDonald et al. (2015)
|
767
|
Nature
|
USA
|
Science & Technology
|
Zhang et al. (2014)
|
607
|
Energy & Environmental Science
|
China
|
Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
|
Rubin et al. (2007)
|
519
|
Energy Policy
|
USA
|
Geochemistry & Geophysics; Mineralogy
|
Benson andCole (2008)
|
491
|
Elements
|
USA
|
Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
|
Presser et al. (2011)
|
460
|
Energy & Environmental Science
|
USA
|
Science & Technology
|
Guan et al. (2008)
|
459
|
Global Environmental Change-Human and Policy Dimensions
|
China
|
Environmental Sciences & Ecology; Geography
|
Zoback andGorelick (2012)
|
434
|
PNAS
|
USA
|
Science & Technology
|
Rubin et al. (2015)
|
432
|
International Journal of Greenhouse Gas Control
|
USA
|
Science & Technology; Energy & Fuels; Engineering
|
Lin et al. (2012)
|
425
|
Nature Materials
|
China
|
Chemistry; Materials Science; Physics
|
Note: TC indicates the total number of citations. |
3.5 Research Hotspots and Topic Clustering Analysis
3.5.1 Research Hotspots
Keywords are the core content of literature research, which can analyze the evolution pattern of research themes, research hotspots, and future directions (Tian et al. 2018)。On the other hand, keyword clustering analysis can present the differences and connections between topics, thus identifying the knowledge communities in a particular research area (Yao et al. 2020). In this paper, through data cleaning and synonym conversion of keywords, and after screening and sorting, the frequency of keywords in the field of CCUS in China and the United States was thus counted and analyzed (Table 5). Table 5 shows the top 15 high-frequency keywords in the field of CCUS in China and the United States during 2000–2021, which reflect the evolution of the thematic pulse of the area over the past 20 years. It can be seen that “CO2 capture” as the keyword of this study appears 528 times in China and 450 times in the United States. It occupies a central and intermediary role. CO2 storage, CO2 emission, flue gas, cost, model, and climate change are also the most frequently reported keywords in China and the United States, which are hot words in the CCUS field. This indicates that the research hotspots in the field of CCUS in both China and the United States show diversity and differentiation, and the variety is reflected in the fact that they involve not only various technical studies but also climate change, application areas, numerical simulation, model construction, cost analysis, and other fields. The differences are reflected in the fact that the Chinese CCUS field emphasizes the application of CO2 utilization technologies in the coal sector. At the same time, the United States shows more attention in the field of CO2-EOR. The United States received the world's first patent for CO2-EOR in 1952 and has been actively deploying the technology worldwide. It also represents the United States' leadership in the field (Llamas et al. 2016). In addition, studies have shown that CO2 utilization is considered an essential factor in driving the future scale-up of CCUS technology (Zhang et al. 2020).
China
|
United States
|
Table 5
Top 15 high-frequency keywords in China and the United States
Rank
|
Keywords
|
Frequency
|
Rank
|
Keywords
|
Frequency
|
1
|
CO2 capture
|
528
|
1
|
CO2 capture
|
450
|
2
|
CO2 storage
|
339
|
2
|
CO2 storage
|
386
|
3
|
Carbon dioxide
|
286
|
3
|
carbon dioxide
|
280
|
4
|
CCS
|
199
|
4
|
CCS
|
229
|
5
|
CO2 emission
|
113
|
5
|
CO2 geological storage
|
123
|
6
|
CO2 geological storage
|
109
|
6
|
climate change
|
107
|
7
|
flue gas
|
108
|
7
|
CO2 emission
|
103
|
8
|
adsorption
|
109
|
8
|
energy
|
100
|
9
|
China
|
94
|
9
|
cost
|
88
|
10
|
model
|
81
|
10
|
technology
|
88
|
11
|
CCUS
|
68
|
11
|
system
|
83
|
12
|
simulation
|
66
|
12
|
flue gas
|
78
|
13
|
energy
|
65
|
13
|
model
|
76
|
14
|
coal
|
58
|
14
|
impact
|
56
|
15
|
cost
|
52
|
15
|
CO2 transport
|
55
|
3.5.2 Topic Clustering Analysis
To better present the research themes in the field of CCUS in China and the United States, this paper uses Citespace software to perform a cluster analysis of Chinese CCUS keywords (Fig. 6). Each cluster is composed of multiple closely related keywords, which are collated to form Table 6 and Table 7. The Q values in Table 6 and Table 7 are greater than 0.3, indicating significant clustering institutions. The S values are greater than 0.7, showing convincing clustering.
Combining Table 6 and Fig. 6a, it can be seen that the thematic clustering in the field of CCUS in China over the past 20 years mainly includes: #0 enhanced gas recovery, #1 coal-fired power plants, #2 dioxide capture, #3 power sector, #4 calcium carbonate, #5 numerical simulation, #6 CO2 absorption, #7 supercritical CO2, #8 chemical looping combustion, #9 life cycle assessment.
Topics #1 and #3 are industries where CCUS technology research is focused on applications. As coal-fired power plants are major carbon emitters, more and more domestic companies are using CCUS technology to address carbon emissions in critical areas, such as the National Energy Group, which has built the largest CCUS complete process demonstration project for coal-fired power plants in China. CCUS technology is superior in reducing emissions in the power industry and is considered one of the essential options for China to achieve profound carbon reduction in the power sector. In the future, CCUS technology will play a more critical role in crucial carbon emissions industries such as power plants, steel, and cement (Fan et al. 2022, Wei et al. 2021).
Topics #2, #4, #6, and #8 are all related to CO2 capture technology, which is the most important technical component of CCUS technology. Depending on the capture mechanism, CO2 capture technology can be divided into several categories: chemical absorption, physical absorption, physical adsorption, membrane separation, deep cooling separation, etc. Chemical absorption and physical absorption methods are relatively the most mature and have been widely used in the chemical industry (Lee &Park 2015, Wilberforce et al. 2021).
Topic #7 mainly deals with research related to carbon dioxide transport. As the pipeline is an economical and convenient transportation mode, it has excellent advantages in carbon dioxide transport of CCUS projects and is also an area of more current research (Lu et al. 2020).
Topics #0, #5, and #9 are standard research methods and application scenarios for CCUS, especially in the CO2 storage and CO2 utilization phase, and are often used to improve CO2 oil recovery rates (Cruz et al. 2021, Haro et al. 2018).
Table 6
Topic clustering and significant keywords in the field of CCUS in China during 2000–2022
Rank
|
Q
|
S
|
Cluster name
|
Cluster name main keywords
|
#0
|
0.82
|
0.91
|
enhanced gas recovery
|
enhanced gas recovery; numerical simulation; permeability; fluid
|
#1
|
0.82
|
0.88
|
coal-fired power plants
|
flue gas; combustion; emission reduction; dissolution; chemical absorption; decomposition; coal phase-out
|
#2
|
0.82
|
0.90
|
dioxide capture
|
gas adsorption; competitive adsorption; sorbent; bituminous coal; natural gas hydrate; methane; nitrogen; membrane
|
#3
|
0.82
|
0.92
|
power sector
|
coal; electricity; adsorbent; coal-ired; power industry; coal gasication; power to gas; energy eiciency; polyeneration system; cogeneration
|
#4
|
0.82
|
0.95
|
calcium carbonate
|
CO2 uptake; pulverized coal; particle size
|
#5
|
0.82
|
0.88
|
numerical simulation
|
CO2 geological storage; CO2-EOR; equation; feasibllity
|
#6
|
0.82
|
0.87
|
CO2 absorption
|
biphasic solvent; absorbent; cyclopentane; ethylenediamine
|
#7
|
0.82
|
0.87
|
supercritical CO2
|
pipeline; CO2 monitoring; carbon dioxide corrosion; corrosion mechanism; pore size distribution
|
#8
|
0.82
|
0.83
|
chemical looping combustion
|
fuel; heat; fluidized bed reactor; pre combustion capture
|
#9
|
0.82
|
1.00
|
life cycle assessment
|
Conversion; CO2 capture and conversion; carbon dioxide utilization; climate
|
Note: Modularity (Q value) indicates the modularity value of the clusters, and it is generally considered that Q > 0.3 means that the clustering structure is significant. Silhouette (S value) indicates the average contour value of clusters, and it is generally considered that S > 0.5 clusters are reasonable, and S > 0.7 means that the clusters are convincing. |
Combined with what is known from Table 7 and Fig. 6b, it can be found that the US CCUS domain theme clusters mainly include: #0 solid sorbent, #1 risk assessment, #2 energy systems, #3 numerical modeling, #4 CO2 capture, #5 climate change, #6 techno-economic analysis, #7 air separation, #8 carbon capture and storage, #9 enhanced oil recovery.
Topic #1 is mainly related to CO2 injection, geological storage, CO2 leakage, and CO2 monitoring. Risk assessment and monitoring of CCUS technology is a critical research task regarding risk assessment before CO2 injection and risk liability issues after long-term storage (Balch &McPherson, 2022).
Topic #0, #4, and #7 are mainly related to CO2 capture technology research. For CO2 capture technology, more and more scholars have begun to research direct air capture technology. This technology can remove CO2 from the air environment using absorbers and is considered a new generation of CO2 capture technology (Madhu et al. 2021, Ozkan et al. 2022).
Topics #3 and #9 contain keywords such as Monte Carlo, Bayesian inference, and CO2-EOR. The current hot area studies simulate and optimize CO2 utilization and geological storage for enhanced recovery of depleted reservoirs using numerical simulation and other methods (Safi et al. 2016).
Topics #2, #5, #6, and #8 mainly include climate change, energy systems, techno-economic analysis, etc. The economic analysis and business model design of CCUS is a hot topic of current research in the field of CCUS and one of the constraints that limit the scale-up of CCUS (Ren et al. 2022, Singh &Colosi 2021, Sullivan et al. 2020).
Based on the differences in the national conditions of the two countries, it can be seen that there are some differences in the clustering of CCUS keyword topics between China and the United States, and the focus of research in the two countries has its emphasis. Therefore, to promote the rapid development of this field, cooperation and communication between the two countries in the field of CCUS technology should be strengthened in the future.
Rank
|
Q
|
S
|
Cluster name main keywords
|
Cluster name main keywords
|
Table 7
Topic clustering and significant keywords in the field of CCUS in the United States during 2000–2022
#0
|
0.77
|
0.88
|
solid sorbent
|
activated carbon; ionic liquid; mesoporous silica; graphene; CO2 capture technology; CO2 adsorption; porous carbon; calcium carbonate
|
#1
|
0.77
|
0.96
|
risk assessment
|
risk analysis; monitoring; CO2 leakage; deep leaming; CO2 injection; risk perception
|
#2
|
0.77
|
0.89
|
energy systems
|
Scenario; climate change mitigation; integrated assessment model; energy transition
|
#3
|
0.77
|
0.91
|
numerical modeling
|
capacity estimation; numerical modeling; monte carlo; bayesian inference
|
#4
|
0.77
|
0.92
|
CO2 capture
|
gas combined cycle; sorbent; direct air capture;
|
#5
|
0.77
|
0.93
|
climate change
|
Climate; energy technology; negative emission technology; carbon management; CO2 mitigation; carbon constraint
|
#6
|
0.77
|
0.86
|
techno-economic analysis
|
economic analysis; technoeconomic analysis; technoeconomic assessment; investment; cost; carbon sequestration cost; technoeconomic assessment
|
#7
|
0.77
|
0.88
|
air separation
|
CO2 adsorption; ionic liquid; solid sorbent; direct air capture
|
#8
|
0.77
|
0.99
|
carbon capture and storage
|
CO2 capture and storage; capital intensive energy technology; system; environmental policy
|
#9
|
0.77
|
0.87
|
enhanced oil recovery
|
CO2-EOR; performance; capacity; CO2 storage efficiency
|
Note: Same as Table 6. |
3.6 Analysis of the temporal evolution of research themes
Time evolution analysis can reveal the development history of the CCUS field, keep abreast of the frontier areas of research, and help grasp future research and development trends in the subject area. In this paper, we use CiteSpace software to map the evolution of keyword co-occurrence time zones, focusing on expressing the interconnection and influence between clusters. The literature information was processed and imported into CiteSpace software to generate a map of the evolution of CCUS time zones in China and the United States, as shown in Fig. 7, to visualize the development of terminology at the frontier of research in the field of CCUS in China and the United States.
As shown in Fig. 7a, from 2004 to 2008, CCUS-related research in China was relatively homogeneous, focusing mainly on CO2 capture and CO2 storage. CCUS-related research in China started as early as 2004 with a larger circle of CO2 capture and storage, indicating that they have been one of the hot topics of research in the field of CCUS until now. CCUS research has grown rapidly during the period 2009–2018. In this period, there are hot spots of study such as CO2 geological storage, CO2 capture and storage, cost, flue gas, supercritical CO2, power plant, system, etc. It is not difficult to find that the research of CCUS has been diversified and interdisciplinary. From 2019 to 2022, with the proposal of China achieving a carbon peak before 2030 and achieving carbon neutrality before 2060, keywords such as carbon neutrality began to appear and have become hot words in the development of the Chinese era. With the future development of crucial carbon-neutral emission reduction technologies, CCUS technology will usher in significant opportunities.
As can be seen from Fig. 7b, during 2004–2008, the field of CCUS in the United States focused on CO2 storage, CO2 capture, CO2 capture and storage, climate change, CO2 emissions, and CO2 transportation during that period. It can be found that the United States research is earlier and more prosperous than that of China. During 2009–2018, the focus started on topics such as life cycle assessment, techno-economic analysis, uncertainty, simulation, supercritical CO2, optimization, leakage, and biomass, which are the hot research topics in the field of CCUS in the United States at that stage. During 2019–2022, the application of machine learning in the field of CCUS has become a focus of attention for US scholars.
It can be seen that although the research hotspots of China and the United States are not entirely the same in different stages. However, both show that the research related to CCUS shows a trend that the research on CCUS theory is becoming more and more systematic, and the depth and breadth of the study are increasing. It has developed from a single technology to full-chain and multidisciplinary research on CCUS. More and more scholars from different disciplinary backgrounds have started to pay attention to and engage in research in this field.
In addition, the CiteSpace software provides an emergent term detection function. Emergent terms refer to terms that appear more often or with higher frequency in a shorter period, and the frontier and trend of the research field can be judged according to the word frequency change of emergent terms, which is suitable for examining emerging trends and sudden changes in the development of disciplines. As shown in Fig. 8. From Fig. 8a, it can be seen that the keyword proliferation point of China's CCUS field research started in 2004, and the change of each keyword proliferation varies. The most vigorous emergent intensity in China is CO2 geological storage, with a strength value of 9.54, which appears more frequently between 2014 and 2017. It indicates that Chinese scholars highly valued this keyword during this period. Secondly, Chinese scholars have received much attention from keywords such as supercritical CO2, numerical simulation, price, uncertainty, and real options. The burst intensity has been maintained at a high level since 2014. However, as CCUS technology evolves and new issues arise, the attention to these keywords has declined. The keywords of stability and deployment will be emphasized from 2020 onwards. It is foreseen that CCUS technology with maturity and strength will be deployed on a large scale in crucial emission reduction industries in the future to achieve the goal of carbon neutrality.
As can be seen from Fig. 8b, the sudden increase of keywords in the CCUS field in the United States began in 2000, earlier than that in China. The most muscular emergent strength is LCA, with a strength value of 5.69, mainly active during 2018–2022. It indicates that this keyword is a crucial area of interest for United States scholars in CCUS. Secondly, the keywords of commercial readiness technology, flue gas, CO2 transportation, renewable energy, and climate change are also the focus of American scholars. The research has been conducted since 2004, and the attention started to decrease until 2020. However, it can be seen that with the continuous development and improvement of CCUS technology, life cycle assessment, negative emission technology, and techno-economic analysis will be the areas that US scholars will focus on in the future.
In conclusion, in the face of intensifying global greenhouse gas emissions, scholars from various countries will pay more and more attention to the R&D and application of CCUS-related technologies, especially the development of new generation technologies and the generation of disruptive technologies. This will significantly promote the development of this technology.