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The resistive switching (RS) mechanism of hybrid organic-inorganic perovskites is an open question until now. Here, a switchable diode-like RS behavior in MAPbBr3 single crystals using Au (or Pt) symmetric electrodes is reported. Both the high resistance state (HRS) and low resistance state (LRS) are electrode-area dependent and light responsive. We propose an electric-field-driven inner p-n junction accompanied by a trap-controlled SCLC conduction mechanism to explain this switchable diode-like RS behavior in MAPbBr3 single crystals.
Keywords
resistive switching, rectifying behavior, hybrid organic-inorganic perovskites, p-n structure
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Posted 04 Dec, 2020
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On 23 Nov, 2020
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On 23 Nov, 2020
Editor invited
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Editorial decision: Major revisions
On 15 Sep, 2020
Review #3 received
Received 13 Sep, 2020
Review #2 received
Received 07 Sep, 2020
Reviewer #3 agreed
On 01 Sep, 2020
Reviewer #2 agreed
On 31 Aug, 2020
Review #1 received
Received 31 Aug, 2020
Reviewers invited
Invitations sent on 30 Aug, 2020
Reviewer #1 agreed
On 30 Aug, 2020
Editor assigned
On 28 Aug, 2020
First submitted
On 27 Aug, 2020
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On 27 Aug, 2020
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On 27 Aug, 2020
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Ceramics
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This preprint is under consideration at Journal of Advanced Ceramics. A preprint is a preliminary version of a manuscript that has not completed peer review at a journal. Research Square does not conduct peer review prior to posting preprints. The posting of a preprint on this server should not be interpreted as an endorsement of its validity or suitability for dissemination as established information or for guiding clinical practice.
Learn more about In Review
Research Article
Badges
Prescreen
This manuscript passed our Prescreen assessment
Complete author information
Appropriate declaration statements
Potential risks to human health
Prescreen
Peer Review Timeline
CURRENT STATUS: Under Review
Version 2
Posted 04 Dec, 2020
No community comments so far
Editor assigned
On 23 Nov, 2020
Submission checks complete
On 23 Nov, 2020
Editor invited
On 23 Nov, 2020
No comments provided
Editorial decision: Major revisions
On 15 Sep, 2020
Review #3 received
Received 13 Sep, 2020
Review #2 received
Received 07 Sep, 2020
Reviewer #3 agreed
On 01 Sep, 2020
Reviewer #2 agreed
On 31 Aug, 2020
Review #1 received
Received 31 Aug, 2020
Reviewers invited
Invitations sent on 30 Aug, 2020
Reviewer #1 agreed
On 30 Aug, 2020
Editor assigned
On 28 Aug, 2020
First submitted
On 27 Aug, 2020
Submission checks complete
On 27 Aug, 2020
Editor invited
On 27 Aug, 2020
Metrics
Comments: 0
PDF Downloads: ...
HTML Views: ...
Subject Areas
Ceramics
License:
This work is licensed under a CC BY 4.0 License. Read Full License
The resistive switching (RS) mechanism of hybrid organic-inorganic perovskites is an open question until now. Here, a switchable diode-like RS behavior in MAPbBr3 single crystals using Au (or Pt) symmetric electrodes is reported. Both the high resistance state (HRS) and low resistance state (LRS) are electrode-area dependent and light responsive. We propose an electric-field-driven inner p-n junction accompanied by a trap-controlled SCLC conduction mechanism to explain this switchable diode-like RS behavior in MAPbBr3 single crystals.
Figure 1
Figure 2
Figure 3
Figure 4
Figure 5
Figure 6
Figure 7
The full text of this article is available to read as a PDF.
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