We studied the optical signature of bipolaron and its effects on the bandgap modulation in the single-layer Transition Metal Dichalcogenides (TMDs) under magnetic field. Using the Huybrecht method, we derived the ground state energies in the modified zero Landau levels for all Fröhlich coupling constants. We take into account both intrinsic longitudinal optical phonon modes and surface optical phonon modes induced by the polar substrate. We observed that the higher the coupling strength, the stronger is the magnetic field effect. The highest amplitude of the bandgap modulation is obtained for the MoS2 monolayer and the lowest with the WSe2 monolayer. We also found that the bipolaron is stable in TMDs. It is seen that the optical absorption presents the threshold values and respectively increases for WSe2, MoSe2, WS2 and MoS2.